Villains who are power hungry seek to obtain more power, be it political, social, physical, supernatural, etc.
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Keith Gremlin
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Cad Spinner
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Calvin Candie
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Camp Bullies
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Captain Frye
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Captain Gutt
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Captain Hook (Disney)
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Carface Carruthers
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Carnegie
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Castor Troy
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Cat R. Waul
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Cell
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Chef
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Chris D'Amico
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Chuck The Evil Sanwich Making Guy
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Cipher
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Cliff Vandercave
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Cobra Commander
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Colonel Miles Quartich
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Commander Red
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Commander Vic Hoskins
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Courtney Shayne
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Cyrus Grissom
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Dagnino
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Darth Maul
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Darth Vader
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Dave (The Penguins of Madagascar)
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David Banner
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David McCall
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Dementors
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Doctor Doom (2005 Film)
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Dolores Umbridge
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Dominic Badguy
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Don Lino
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Dooku
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Douche
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Dr Evil
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Dr Zachary Smith
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Dr Zander Rice
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Dr. Frank-N-Furter
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Dr. Julius No
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Dr. Porkchop
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Dr. Robotnik (2020 Film)
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Draco Malfoy
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Drago Bludvist
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Drago's Bewilderbeast
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Dragon (Sleeping Beauty)
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Drake
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Duke of Weselton
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Gallian
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Gargamel
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Garlic Jr
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Garmadon (The Lego Ninjago Movie)
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Gaston Legume
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Gazeem
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General Grievous
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General Hux
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General Katana
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General Mandible
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General Shanker
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General Zod
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Gilderoy Lockhart
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Gill-Man
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Goblin Queen
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Godzilla
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Gorilla Grodd (DC Animated Universe)
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Governor Ratcliffe
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Grand Moff Tarkin
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Grandmaster
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Green Goblin
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Grima Wormtongue
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Grizzly Bear (Dawn of the Planet of the Apes)
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Lady Tremaine (2015)
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Lawrence Van Dough
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Leatherface
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Leon Rom
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Leopard Seal (Happy Feet)
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Lex Luthor (Christopher Reeve Superman Films)
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Lex Luthor (DC Extended Universe)
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Lex Luthor (Superman Returns)
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Linus
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Lizard
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Loki Laufeyson (Marvel Cinematic Universe)
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Lord Business
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Lord Cutler Beckett
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Lord Dargis
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Lord Farquaad
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Lord Henry Blackwood
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Lord Maliss